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The PUREX process was invented by Herbert H. Anderson and Larned B. Asprey at the Metallurgical Laboratory at the University of Chicago, as part of the Manhattan Project under Glenn T. Seaborg; their patent "Solvent Extraction Process for Plutonium" filed in 1947, [14] mentions tributyl phosphate as the major reactant which accomplishes the ...
PUREX, the current standard method, is an acronym standing for Plutonium and Uranium Recovery by EXtraction. The PUREX process is a liquid-liquid extraction method used to reprocess spent nuclear fuel, to extract uranium and plutonium, independent of each other, from the fission products. This is the most developed and widely used process in ...
The first reprocessing approach is based on the PUREX (Plutonium Uranium Reduction EXtraction) process, which is the standard and mature technology applied worldwide to recover uranium and plutonium from spent nuclear fuel at industrial scale. Following the dissolution of the spent fuel in nitric acid and the removal of uranium and plutonium ...
The most common reprocessing technique, PUREX, presents a particular concern since it was expressly designed to separate plutonium. Early proposals for the breeder-reactor fuel cycle posed an even greater proliferation concern because they would use PUREX to separate plutonium in a highly attractive isotopic form for use in nuclear weapons. [50 ...
A significant amount of zirconium is formed by the fission process; some of this consists of short-lived radionuclides (95 Zr and 97 Zr which decay to molybdenum), while almost 10% of the fission products mixture after years of decay consists of five stable or nearly stable isotopes of zirconium plus 93 Zr with a halflife of 1.53 million years ...
It is also used in nuclear reprocessing as part of the PUREX process. A 15–40% (usually about 30%) solution of tributyl phosphate in kerosene or dodecane is used in the liquid–liquid extraction (solvent extraction) of uranium, plutonium, and thorium from spent uranium nuclear fuel rods dissolved in nitric acid. Liquid extraction can also be ...
It is possible, however, to remove the americium from the plutonium by a chemical separation process. Even under the worst conditions, the americium/plutonium mixture is less radioactive than a spent-fuel dissolution liquor, so it should be relatively straightforward to recover the plutonium by PUREX or another aqueous reprocessing method.
Phase diagram of neptunium α-neptunium takes on an orthorhombic structure, resembling a highly distorted body-centered cubic structure. [ 13 ] [ 14 ] Each neptunium atom is coordinated to four others and the Np–Np bond lengths are 260 pm. [ 15 ] It is the densest of all the actinides and the fifth-densest of all naturally occurring elements ...