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Pump–probe microscopy is a non-linear optical imaging modality used in femtochemistry to study chemical reactions. It generates high-contrast images from endogenous non-fluorescent targets. It generates high-contrast images from endogenous non-fluorescent targets.
Cartoon of the pump-probe spectroscopy approach. The sample is first prepared in an excited state by a laser pulse and then probed by an X-ray pulse. With the advent of XFELs, sources that can provide extremely brilliant (more than five orders of magnitude larger than synchrotron sources) and extremely short X-ray pulses, X-ray spectroscopies ...
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When the electron dynamics in the bound states just above the Fermi level need to be studied, two-photon excitation in pump-probe setups is used. There, the first photon of low-enough energy is used to excite electrons into unoccupied bands that are still below the energy necessary for photoemission (i.e. between the Fermi and vacuum levels).
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In physics and physical chemistry, time-resolved spectroscopy is the study of dynamic processes in materials or chemical compounds by means of spectroscopic techniques.Most often, processes are studied after the illumination of a material occurs, but in principle, the technique can be applied to any process that leads to a change in properties of a material.
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